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Carlo Maria Francesco d'Assisi Pasquale Ferdinando Antonio di Padova Francesco de Paola Alfonso Andrea Avelino Tancredi di Borbone delle Due Sicilie was born 10 November 1870 in Gries am Brenner, Innsbruck-Land District, Tyrol, Austria to Alfonso di Borbone delle Due Sicilie (1841-1934) and Maria Antonietta di Borbone delle Due Sicilie (1851-1938) and died 11 November 1949 Seville, Province of Seville, Andalusia, Spain of unspecified causes. He married María de las Mercedes de España (1880-1904) 14 February 1901 in Madrid, Spain. He married Louise d'Orléans (1882-1958) 16 November 1907 in Wood Norton, Worcestershire, England, United Kingdom.
Children
| Name | Birth | Death | Joined with |
| Alfonso di Borbone delle Due Sicilie (1901-1964) | 30 November 1901 Madrid, Spain | 3 February 1964 Vienna, Austria | Alice di Borbone-Parma (1917-2017) |
| Fernando di Borbone delle Due Sicilie (1903-1905) | 6 March 1903 Madrid, Spain | 4 August 1905 San Sebastián, Gipuzkoa, Basque Country, Spain | |
| Isabella Alfonsa di Borbone delle Due Sicilie (1904-1985) | 16 October 1904 Madrid, Spain | 18 July 1985 Madrid, Spain | Jan Kanty Zamoyski h. Jelita (1900-1961) |
| Name | Birth | Death | Joined with |
| Carlo di Borbone delle Due Sicilie (1908-1936) | 5 September 1908 Santander, Cantabria, Spain | 27 September 1936 Elgoibar, Gipuzkoa, Basque Country, Spain | |
| Maria de los Dolores di Borbone delle Due Sicilie (1909-1996) | 15 September 1909 Madrid, Poland | 11 May 1996 Madrid, Spain | August Czartoryski (1907-1946) Carlos Chias Osorio (1925-) |
| María Mercedes di Borbone delle Due Sicilie (1910-2000) | 23 December 1910 Madrid, Spain | 2 January 2000 Lanzarote, Canary Islands, Spain | Juan, Conde de Barcelona (1913-1993) |
| Maria de la Esperanza di Borbone delle Due Sicilie (1914-2005) | 14 June 1914 Madrid, Spain | 8 October 2005 Villamanrique de la Condesa, Province of Seville, Andalusia, Spain | Pedro de Alcântara de Orléans (1913-2007) |